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전임교원이 최근 5년간 출판한 논문 중, 연도별 카테고리별 피인용 상위 1%에 달성된 논문
매월 1회 업데이트

SCIE Article

Unveiling dual-linkage 3D hexaiminobenzene metal-organic frameworks towards long-lasting advanced reversible Zn-air batteries

Author

Shinde, Sambhaji S.; Lee, Chi Ho; Jung, Jin-Young; Wagh, Nayantara K.; Kim, Sung-Hae; Kim, Dong-Hyung; Lin, Chao; Lee, Sang Uck; Lee, Jung-Ho;

Corresponding Author Info

Prof. Lee, Sang Uck (바이오나노학과 이상욱 교수)

Professor

E-mail

sulee@hanyang.ac.kr

Document Type

Source

ENERGY & ENVIRONMENTAL SCIENCE 2019, 12, 2, 727-738

Times Cited

141 (2022.2.21.)

External Information

https://doi.org/10.1039/C8EE02679C

Abstract

[History]
- 11월/12월 2019부로, 이 인용 빈도가 높은 논문의 인용 횟수가 분야와 출판 연도에 대해 인용 빈도가 높은 임계값을 기반으로 Chemistry 관련 학술 분야에서 상위 1%에 올랐습니다.

[Abstract]
Advanced Zn-air batteries (ZABs) with ultrahigh cycle life, which also harness energy with bifunctional electrochemical reactions, are significantly challenging for the commercialization of hybrid/electric vehicles and wearable electronics. Herein, we demonstrated robust aqueous and flexible ZABs with novel three-dimensional dual-linked hexaiminobenzene metal-organic framework (Mn/Fe-HIB-MOF)-based bifunctional oxygen electrocatalysts and superionic functionalized bio-cellulose electrolytes (64 mS cm(-1)). The well-defined quintet-shelled hollow sphere MOFs possess a hierarchical porous structure, excellent packing density with a surface area of 2298 m(2) g(-1), and chemical stability as compared to conventional MOFs. Mn/Fe-HIB-MOF exhibited superior bifunctional oxygen electrocatalytic activity (0.627 V) with half-wave potential (0.883 V) for oxygen reduction and overpotential (280 mV@10 mA cm(-2)) for oxygen evolution reactions, outperforming commercial Pt/C and RuO2. Their favorable oxygen reactions and surface electronic structures were confirmed by density functional theory. Significantly, the Mn/Fe-HIB-MOF cathode demonstrated the highest lifetimes reported to date for rechargeable ZABs, namely 1000 h (0.75 V voltage gap@10 mA cm(-2)) over 6000 cycles and 600 h (efficiency approximate to 65.24%@25 mA cm(-2)) over 3600 cycles with excellent flexibility for liquid and all-solid-state flexible ZABs, respectively. These promising results illustrate the great potential of these novel hexaiminobenzene MOFs and superionic bio-cellulose membranes for the commercial implementation of rechargeable ZABs.

Web of Science Categories

Chemistry, Multidisciplinary; Energy & Fuels; Engineering, Chemical; Environmental Sciences

Funding

Language

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